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Ruthenium-catalyzed C–H bond functionalization in cascade and one-pot transformations

Abstract : Ruthenium complexes are well known as remarkable pre-catalysts for challenging C-H bond functionalizations. Combining them with other types of chemical reactions in a tandem or one-pot fashion is appealing from a sustainable point of view because it gives access to new strategies to diminish steps devoted to purification and isolation of (sometimes unstable) intermediates. This non-exhaustive review highlights the different approaches enabling these technologies with a particular focus on the understanding for the compatibility of the different reaction sequences. More precisely, ruthenium-catalyzed C-H bond functionalization turned out to be compatible with several organic transformations, metal-mediated reactions and transition metal catalysis. Graphical abstract Highlights-Ruthenium complexes are compatible with one-pot and tandem transformations involving C-H bond functionalization.-Ruthenium-catalyzed C-H bond functionalization has been successfully coupled with other C-H bond functionalization reactions.-Different organic and metal-mediated transformations operate in a concerted manner with ruthenium-catalyzed C-H bond functionalization.-The merger of ruthenium-catalyzed C-H bond functionalization strategies with several transition metal catalysis is attractive for green chemistry and sustainable approaches. Ru catalysis C-H bond functionalization metal catalysis organic reactions cascade and one-pot substrates products metal meditated
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https://hal.archives-ouvertes.fr/hal-02989137
Contributeur : Rafael Gramage-Doria <>
Soumis le : jeudi 5 novembre 2020 - 09:27:31
Dernière modification le : mardi 12 janvier 2021 - 16:38:02

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Rafael Gramage-Doria, Christian Bruneau. Ruthenium-catalyzed C–H bond functionalization in cascade and one-pot transformations. Coordination Chemistry Reviews, Elsevier, 2021, 428, pp.213602. ⟨10.1016/j.ccr.2020.213602⟩. ⟨hal-02989137⟩

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